Journal article
Nano letters, 2016
APA
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Rösner, M., Steinke, C., Lorke, M., Gies, C., Jahnke, F., & Wehling, T. (2016). Two-Dimensional Heterojunctions from Nonlocal Manipulations of the Interactions. Nano Letters.
Chicago/Turabian
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Rösner, M., C. Steinke, M. Lorke, C. Gies, F. Jahnke, and T. Wehling. “Two-Dimensional Heterojunctions from Nonlocal Manipulations of the Interactions.” Nano letters (2016).
MLA
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Rösner, M., et al. “Two-Dimensional Heterojunctions from Nonlocal Manipulations of the Interactions.” Nano Letters, 2016.
BibTeX Click to copy
@article{m2016a,
title = {Two-Dimensional Heterojunctions from Nonlocal Manipulations of the Interactions.},
year = {2016},
journal = {Nano letters},
author = {Rösner, M. and Steinke, C. and Lorke, M. and Gies, C. and Jahnke, F. and Wehling, T.}
}
We propose to create lateral heterojunctions in two-dimensional materials based on nonlocal manipulations of the Coulomb interaction using structured dielectric environments. By means of ab initio calculations for MoS2 as well as generic semiconductor models, we show that the Coulomb interaction-induced self-energy corrections in real space are sufficiently nonlocal to be manipulated externally, but still local enough to induce spatially sharp interfaces within a single homogeneous monolayer to form heterojunctions. We find a type-II heterojunction band scheme promoted by a laterally structured dielectric environment, which exhibits a sharp band gap crossover within less than 5 unit cells.